Award Abstract # 1339264
Tropospheric Anthropogenic Aerosols and Climate

NSF Org: AGS
Division of Atmospheric and Geospace Sciences
Recipient: MASSACHUSETTS INSTITUTE OF TECHNOLOGY
Initial Amendment Date: November 6, 2013
Latest Amendment Date: November 6, 2013
Award Number: 1339264
Award Instrument: Standard Grant
Program Manager: Ming Cai
AGS
 Division of Atmospheric and Geospace Sciences
GEO
 Directorate for Geosciences
Start Date: December 1, 2013
End Date: November 30, 2017 (Estimated)
Total Intended Award Amount: $600,000.00
Total Awarded Amount to Date: $600,000.00
Funds Obligated to Date: FY 2014 = $600,000.00
History of Investigator:
  • Chien Wang (Principal Investigator)
    wangc@mit.edu
Recipient Sponsored Research Office: Massachusetts Institute of Technology
77 MASSACHUSETTS AVE
CAMBRIDGE
MA  US  02139-4301
(617)253-1000
Sponsor Congressional District: 07
Primary Place of Performance: Massachusetts Institute of Technology
77 Massachusetts Ave
Cambridge
MA  US  02129-4307
Primary Place of Performance
Congressional District:
07
Unique Entity Identifier (UEI): E2NYLCDML6V1
Parent UEI: E2NYLCDML6V1
NSF Program(s): Atmospheric Chemistry,
Physical & Dynamic Meteorology,
Climate & Large-Scale Dynamics
Primary Program Source: 01001415DB NSF RESEARCH & RELATED ACTIVIT
Program Reference Code(s): 0000, 4444, OTHR
Program Element Code(s): 152400, 152500, 574000
Award Agency Code: 4900
Fund Agency Code: 4900
Assistance Listing Number(s): 47.050

ABSTRACT

This project focuses on addressing three critical science issues regarding aerosol climate forcing, response, and feedback: (1) the impacts of carbonaceous mixtures on the formation and radiation of water and ice clouds in addition to the direct radiative forcing of aerosols; (2) the climate responses reflected in the changes of clouds and precipitation caused by anthropogenic aerosols through both optical-dynamical (direct) and cloud microphysical (indirect) connections; and (3) the nonlinear effects arising from the coexistence of non-uniformly distributed anthropogenic aerosols and relatively well-distributed greenhouse gases, and from the coexistence of absorbing and scattering aerosols. To address these science issues, the PI and his team will specifically improve three aspects of our aerosol-climate model: (1) the formation, physiochemical conversion, and optical properties of carbonaceous aerosols; (2) the treatment of cloud processing and recycling of carbonaceous contents through cloud and precipitation evaporation; and (3) the impacts of anthropogenic aerosols particularly carbonaceous mixtures on ice nucleation.

These improvements with designed long ensemble integrations and special sensitivity simulations would enable the study of several key but still poorly described processes in the models, and thus to better understand the climate responses to anthropogenic aerosols both through the direct and indirect effects. The model developed by this program will be provided to the community after the completion of the project, as a unique option to the current CESM aerosol models, for conducting climate response/feedback study with a size- and mixing state-dependent aerosol representation and a good computationally efficiency. Thus the broader impacts of the project are high.

PUBLICATIONS PRODUCED AS A RESULT OF THIS RESEARCH

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(Showing: 1 - 10 of 24)
Cohen, J. B., and C. Wang "Estimating global black carbon emissions using a top-down Kalman filter approach" J. Geophys. Res. , v.119 , 2014 , p.307 10.1002/2013JD019912
Cohen, J. B., and C. Wang "Estimating global black carbon emissions using a top-down Kalman filter approach" J. Geophys. Res. , v.119 , 2014 , p.307 10.1002/2013JD019912
Cziczo, D. J. and K. D. Froyd "Sampling the composition of cirrus ice residuals" Atmospheric Research , v.142 , 2014 , p.15
Cziczo, D. J. and K. D. Froyd, "Sampling the composition of cirrus ice residuals" Atmos. Res. , v.142 , 2014 , p.15
Garimella, S., D. A. Rothenberg, M. J. Wolf, C. Wang, and D. J. Cziczo "¬How uncertainty in field measurements of ice nucleating particles influences modeled cloud forcing" J. Atmos. Sci. , v.75 , 2018 , p.179 10.1175/JAS-D-17-0089.1
Garimella, S., D. A. Rothenberg*, M. J. Wolf, R. O. David, Z. A. Kanji, C. Wang, M. Rösch, and D. J. Cziczo "Uncertainty in counting ice nucleating particles with continuous flow diffusion chambers" Atmospheric Chemistry and Physics , v.17 , 2017 , p.10855 10.5194/acp-17-10855-2017
Grandey, B., H. Cheng, and C. Wang "Transient climate impacts for scenarios of aerosol emissions from Asia: a story of coal versus gas" J. Climate , v.29 , 2016 , p.284 10.1175/JCLI-D-15-0555.1
Grandey, B. S., and C. Wang "Enhanced marine sulphur emissions offset global warming and impact rainfall" Scientific Report , v.5 , 2015 , p.13055 10.1038/srep13055
Grandey, B. S., and C. Wang "Enhanced marine sulphur emissions offset global warming and impact rainfall" Scientific Reports , v.5 , 2015 , p.13055 (20 10.1038/srep13055
Grandey, B. S., H. Cheng, and C. Wang "Transient climate impacts for scenarios of aerosol emissions from Asia: a story of coal versus gas" Journal of Climate , v.29 , 2016 , p.2849 10.1175/JCLI-D-15-0555.1
Grandey, B. S., H.-H. Lee, and C. Wang "Radiative effects of inter-annually varying versus inter-annually invariant aerosol emissions from fires" Atmos. Chem. Phys. , v.16 , 2016 , p.14495 10.5194/acp-16-14495-2016
(Showing: 1 - 10 of 24)

PROJECT OUTCOMES REPORT

Disclaimer

This Project Outcomes Report for the General Public is displayed verbatim as submitted by the Principal Investigator (PI) for this award. Any opinions, findings, and conclusions or recommendations expressed in this Report are those of the PI and do not necessarily reflect the views of the National Science Foundation; NSF has not approved or endorsed its content.

Aerosol remains one of the most uncertain factors in projecting climate, much owing to the sophisticated feedbacks involved in the interplays between aerosol and clouds and the difficulty in representing these processes in climate models. This project is to study these critical but still poorly understood science issues. Our achievements in research are primarily on: (a) advancing our knowledge; and (b) developing and producing the state-of-art computational tools and laboratory as well as field results to improve the representations of aerosol-cloud processes in climate models.

 

In advancing knowledge of aerosol-cloud interaction and it’s impacts on climate, our researches have produced many unique results and first-time findings, which are mostly published with a few still under review or to be submitted soon. These research findings could advance the frontier of our science and also have broader impacts on other science fields and the processes of making effective climate and environment mitigation policies. Here are several examples:

  1. Using a large quantity of climate model results alongside observational data, we have revealed the dominant role of aerosol in determining the changing pattern of large-scale precipitation in the past, and indicated the importance for models to have physically-based representation of aerosol-cloud processes in order to reproduce observed precipitation trend.
  2. We have extensively studied the influence of aerosols on the monsoons. Detailed modeling analyses have been conducted to examine various hypotheses about this effect and revealed a mechanism that soil moisture could preserve the memory of aerosol forcing in monsoon onset stage through deep monsoon stage.
  3. Our recent work has identified a reversal of Indian summer monsoon rainfall since 2002 from a half-century-long drying to persistent wetting, that is opposite to many previous projections of the continuation of the long lasting drying trend. This important finding, however, raises a serious issue about the abrupt warming over Indian land area in recent decade that is found to behind this reversal, and suggests to propose new ideas regarding anthropogenic forcings including those of aerosols in causing such a change.
  4. Another direction our research has made significant progress is about the climate impacts of biomass burning emitted aerosols. Our work suggests a substantial year-to-year variation of biomass burning emissions and using a simple average across multiple years, as adopted in many modeling efforts, would substantially overestimated the cooling effect of this type of aerosols. Specifically regarding frequent biomass burning activities in Southeast Asia, we have, for the first time, calculated contribution of biomass burning in comparison to that of other non-fire combustions to the worsening of air quality in that region based on observations and modeling results.
  5. Our study on the potential climate outcome of energy usages in Asia suggests a significant impact on both regional and global precipitation distribution by an extensive coal usage in Asia.
  6. We have also examined the geoengineering proposal of ocean fertilization to decrease atmospheric CO2 concentration, and found such practice could lead to adverse climate outcome particularly of precipitation distribution.

 

To assist above research efforts, we have also developed several novel modeling and data science methods. These including new methods to simulate the formation of cloud droplets or ice crystals from aerosols We have also developed the first-ever inverse modeling platform to use observational data for optimizing our estimate of black carbon emissions. Many of these have been used to improve the Multi-modal, 2-Moment, Mixing-resolving Aerosol model for Climate Research or MARC that has been coupled with NCAR-DOE Community Earth System Model CESM. MARC-CESM with improved schemes has been evaluated extensively against observations and other aerosol modules, and also used to examine the importance of many of these advancements in process-representation. 

 

Our team members have presented the research findings in various scientific conferences, published many peer reviewed papers, and joined communication with governments, policy-making bodies, and general public. We have published three review articles for broader communities. The aerosol model MARC developed in this project has been released in public domain. The project has also produced datasets of long-term simulations designed for examining climate responses to various aerosol configurations. These will be made available to interesting parties following the data management plan.

 


Last Modified: 01/12/2018
Modified by: Chien Wang

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