Award Abstract # 1104642
Measurements of Total Water on the Gulfstream-V for Deep Convective Clouds and Chemistry (DC3)

NSF Org: AGS
Division of Atmospheric and Geospace Sciences
Recipient: THE REGENTS OF THE UNIVERSITY OF COLORADO
Initial Amendment Date: December 8, 2011
Latest Amendment Date: January 16, 2014
Award Number: 1104642
Award Instrument: Continuing Grant
Program Manager: Nicholas Anderson
nanderso@nsf.gov
 (703)292-4715
AGS
 Division of Atmospheric and Geospace Sciences
GEO
 Directorate for Geosciences
Start Date: January 1, 2012
End Date: December 31, 2016 (Estimated)
Total Intended Award Amount: $374,112.00
Total Awarded Amount to Date: $374,112.00
Funds Obligated to Date: FY 2012 = $179,955.00
FY 2013 = $94,013.00

FY 2014 = $100,144.00
History of Investigator:
  • Darin Toohey (Principal Investigator)
    toohey@colorado.edu
  • Linnea Avallone (Former Principal Investigator)
Recipient Sponsored Research Office: University of Colorado at Boulder
3100 MARINE ST
Boulder
CO  US  80309-0001
(303)492-6221
Sponsor Congressional District: 02
Primary Place of Performance: University of Colorado at Boulder
3100 MARINE ST
Boulder
CO  US  80309-0001
Primary Place of Performance
Congressional District:
02
Unique Entity Identifier (UEI): SPVKK1RC2MZ3
Parent UEI:
NSF Program(s): Physical & Dynamic Meteorology
Primary Program Source: 01001314DB NSF RESEARCH & RELATED ACTIVIT
01001213DB NSF RESEARCH & RELATED ACTIVIT

01001415DB NSF RESEARCH & RELATED ACTIVIT
Program Reference Code(s): 0000, OTHR
Program Element Code(s): 152500
Award Agency Code: 4900
Fund Agency Code: 4900
Assistance Listing Number(s): 47.050

ABSTRACT

Combined influences of water vapor, ozone, aerosols and cirrus clouds in the upper-troposphere/lower-stratosphere (UTLS) region serve to strongly modulate radiative forcing of the earth's climate system. The composition of this region is affected not only by chemical processes, but also by dynamical ones such as cross-tropopause exchange and convective transports originating near the earth's surface. The Deep Convective Clouds and Chemistry (DC3) field campaign, to be conducted May-June 2012, will support study of the contrasting impacts of continental midlatitude thunderstorm systems on UTLS composition and chemistry within three regions (viz. northeastern Colorado, western Oklahoma and Texas, and northern Alabama) characterized by differing background chemistry and characteristic storm behavior. This award will support adaptation of an existing tunable diode laser-based instrument, the University of Colorado closed-path laser hygrometer, to make measurements of total water (from which condensed liquid and ice water contents may be derived) aboard the NSF/NCAR GV research aircraft during DC3. A new inlet specific to the selected sampling location aboard the GV will be designed and built in collaboration with a consultant from Embry-Riddle Aeronautical University to enable accurate sampling of a wide range of cloud particle sizes (10-400 micrometers).

The intellectual merit of this research rests on provision of precise and accurate measurements of total water at high spatial resolution within the upper reaches of midlatitude convective cloud systems, which will in-turn allow investigators to describe differing transport properties of shear-driven vs. airmass-type thunderstorms, their attendant evolving microphysical properties over cloud lifecycles, and how anvil radiative environments differ from region to region and with time during the interval 12-48 hours after cessation of active convection. Broader impacts will include graduate student training and public outreach, but will ultimately extend to improved understanding of controls on atmospheric ozone and associated links to climate assessment and policy formulation.

PUBLICATIONS PRODUCED AS A RESULT OF THIS RESEARCH

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A. Mukherjee and D.W. Toohey "A study of aerosol properties based on observations of particulate matter from the U.S. Embassy in Beijing, China" Earth's Future , v.4 , 2016 , p.381 doi:10.1002/2016EF000367
C.H. Twohy, G.R. McMeeking, P.J. DeMott, C.S. McCluskey, T.C.J. Hill, S.M. Burrows, G.R. Kulkarni, M. Tanarhte, D.N. Kafle, andD.W. Toohey "Abundance of fluorescent biological aerosol particles at temperatures conducive to the formation of mixed-phase and cirrus clouds." Atmos. Chem. Phys. , v.16 , 2016 , p.8205 doi:10.5194/acp-16-8205-2016.
J.L. Stith, L. Avallone, A. Bansemer, B. Basarab, S.W. Dorsi, B. Fuchs, R.P. Lawson, D.C. Rogers, S. Rutledge, and D.W. Toohey "Ice particles in the upper anvil regions of mid-latitude continental thunderstorms: The case for frozen-drop aggregates" Atmos. Chem. Phys. , v.14 , 2014 , p.1973 10.5194/acp-14-1973-2014
J.L. Stith, L. Avallone, A. Bansemer, B. Basarab, S.W. Dorsi, B. Fuchs, R.P. Lawson, D.C. Rogers, S. Rutledge, and D.W. Toohey "Ice particles in the upper anvil regions of mid-latitude continental thunderstorms: The case for frozen-drop aggregates" Atmospheric Chemistry and Physics , v.14 , 2014 , p.1973 10.5194/acp-14-1973-2014
S. Dorsi, L. Kalnajs, D. Toohey, and L. Avallone "A Fiber-Coupled Laser Hygrometer for Airborne Total Water Measurements" Atmos. Meas. Tech. , v.7 , 2014 , p.215 10.5194/amt-7-215-2014
S. Dorsi, L. Kalnajs, D. Toohey, and L. Avallone "A Fiber-Coupled Laser Hygrometer for Airborne Total Water Measurements" Atmospheric Measurement Techniques , v.7 , 2014 , p.215 10.5194/amt-7-215-2014

PROJECT OUTCOMES REPORT

Disclaimer

This Project Outcomes Report for the General Public is displayed verbatim as submitted by the Principal Investigator (PI) for this award. Any opinions, findings, and conclusions or recommendations expressed in this Report are those of the PI and do not necessarily reflect the views of the National Science Foundation; NSF has not approved or endorsed its content.

A new laser-based instrument to measure cloud-water was developed and flown on the Gulfstream-V National Science Foundation aircraft during multiple field campaigns. By rapidly warming the air sampled by a foward-facing inlet, the instrument evaporates water and subsequently measures the total amount of water vapor, allowing for the determination of the amount of condensed water in clouds. This quantity is important for understanding cloud formation, precipitation, and interactions of clouds with visible and infrared radiation. In conjunction with other observations, the results of these studies allow for the identification and characterization of different types of particles in clouds. For example, in one publication it was shown that at the tops of thunderstorms there is a type of particle called a "frozen droplet aggregate", essentially a twisted, long chain of droplets that stick together upon freezing, a process that is faciltated by electric charges created by lightning in thunderstorms. In addition to the observations in and around thunderstorms in the continental United States, observations were obtained in the Southern Hemisphere near Antarctica in "mixed-phased clouds," or clouds containing both liquid and frozen water in the same space. These clouds are particularly difficult to model; therefore, observations directly within them help to constrain models that are used to predict the impacts of such clouds on precipitation and energy exchange near the earth's surface. Finally, we were able to obtain the first observations of cloudwater contents from a research aircraft flying over a highly polluted region in the western Pacific Ocean. These observations will allow future studies into the role of natural and human-caused sources of particulates on cloud properties. Specifically, there is an interest in quantifying a phenomenon called the "aerosol indirect effect," or how particle enhancements supress the sizes of cloud droplets which in turn reduces precipitation back to the surface. Studies such as these are useful for determining the impact of air pollution on rainfall patterns, something that is important for agriculture as well as human health.


Last Modified: 03/31/2017
Modified by: Darin W Toohey

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