Award Abstract # 0830916
Collaborative Research: Improving Estimated Fluxes of Greenhouse Gases over North America Using a Receptor-Oriented Modeling Framework and In-situ Atmospheric Measurements

NSF Org: AGS
Division of Atmospheric and Geospace Sciences
Recipient: PRESIDENT AND FELLOWS OF HARVARD COLLEGE
Initial Amendment Date: December 3, 2008
Latest Amendment Date: February 4, 2011
Award Number: 0830916
Award Instrument: Continuing Grant
Program Manager: William (Bill) C. Keene
AGS
 Division of Atmospheric and Geospace Sciences
GEO
 Directorate for Geosciences
Start Date: January 1, 2009
End Date: December 31, 2011 (Estimated)
Total Intended Award Amount: $216,000.00
Total Awarded Amount to Date: $216,000.00
Funds Obligated to Date: FY 2009 = $72,000.00
FY 2010 = $72,000.00

FY 2011 = $72,000.00
History of Investigator:
  • Steven Wofsy (Principal Investigator)
    swofsy@seas.harvard.edu
Recipient Sponsored Research Office: Harvard University
1033 MASSACHUSETTS AVE STE 3
CAMBRIDGE
MA  US  02138-5366
(617)495-5501
Sponsor Congressional District: 05
Primary Place of Performance: Harvard University
1033 MASSACHUSETTS AVE STE 3
CAMBRIDGE
MA  US  02138-5366
Primary Place of Performance
Congressional District:
05
Unique Entity Identifier (UEI): LN53LCFJFL45
Parent UEI:
NSF Program(s): Atmospheric Chemistry
Primary Program Source: 01000910DB NSF RESEARCH & RELATED ACTIVIT
01001011DB NSF RESEARCH & RELATED ACTIVIT

01001112DB NSF RESEARCH & RELATED ACTIVIT
Program Reference Code(s): 0000, OTHR
Program Element Code(s): 152400
Award Agency Code: 4900
Fund Agency Code: 4900
Assistance Listing Number(s): 47.050

ABSTRACT

The work aims to establish accurate top-down estimates of the surface sources and sinks for important greenhouse gases, including carbon dioxide (CO2), methane (CH4), nitrous oxide (N2O), and carbon monoxide (CO) over North America, and address individual science questions, particularly with regard to the causes of variability on diurnal, seasonal, and interannual timescales that underlie these estimates. Collocated airborne and tower-based measurements of these gases for selected months in the period 2003-2011 will be analyzed using a receptor-oriented Lagrangian particle dispersion model driven by a version of the Weather Research and Forecasting (WRF) model adapted to flux inversion work. The analysis will provide an assessment tool for independent bottom-up emission estimates from existing inventories. The availability of reliable transport fields and a conjoint analysis of the four gases will be critical to the success of the study.

Human-induced changes in atmospheric concentrations of greenhouse gases are a major societal concern discussed in the press, in Congress, and by ordinary citizens every day. Currently there is no validation for inventory-based estimates of U.S. and North American contributions to this global problem, and there are indications that these estimates may be in error.

The work will decisively improve this situation by providing new assessments based on strong physical and observational constraints. The data, results, and software will be made publicly available during the research, and the principal investigators will engage in public outreach by communicating the results that are pertinent to the public debate on climate change.

PUBLICATIONS PRODUCED AS A RESULT OF THIS RESEARCH

Note:  When clicking on a Digital Object Identifier (DOI) number, you will be taken to an external site maintained by the publisher. Some full text articles may not yet be available without a charge during the embargo (administrative interval).

Some links on this page may take you to non-federal websites. Their policies may differ from this site.

Kort, EA; Eluszkiewicz, J; Stephens, BB; Miller, JB; Gerbig, C; Nehrkorn, T; Daube, BC; Kaplan, JO; Houweling, S; Wofsy, SC "Emissions of CH4 and N2O over the United States and Canada based on a receptor-oriented modeling framework and COBRA-NA atmospheric observations" GEOPHYSICAL RESEARCH LETTERS , v.35 , 2008 View record at Web of Science 10.1029/2008GL03403
Lin, JC; Pejam, MR; Chan, E; Wofsy, SC; Gottlieb, EW; Margolis, HA; McCaughey, JH "Attributing uncertainties in simulated biospheric carbon fluxes to different error sources" GLOBAL BIOGEOCHEMICAL CYCLES , v.25 , 2011 View record at Web of Science 10.1029/2010GB00388
Mahadevan, P.; Wofsy, S. C. ; Matross, D. M.; Xiao,X. ;Dunn, A. L. ; Lin, J. C. ; Gerbig,C. ; Munger, J. W. ; Chow,V. Y. ; Gottlieb, E. W. "A satellite-based biosphere parameterization for net ecosystem CO2 exchange: Vegetation Photosynthesis and Respiration Model (VPRM)" Global biogeochemical cycles , 2008 10.1029/2006GB002735
McKain K.;Wofsy S; Nehrkorn T.; Eluszkiewicz J; Ehleringer J; Stephens B "Assessment of ground-based atmospheric observations for verification of greenhouse gas emissions from an urban region" Proceedings of the National Academy of Sciences , 2012 doi 10.1073/pnas.1116645109
Miller, SM; Kort, EA; Hirsch, AI; Dlugokencky, EJ; Andrews, AE; Xu, X; Tian, H; Nehrkorn, T; Eluszkiewicz, J; Michalak, AM; Wofsy, SC "Regional sources of nitrous oxide over the United States: Seasonal variation and spatial distribution" JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES , v.117 , 2012 View record at Web of Science 10.1029/2011JD01695
Nehrkorn, T; Eluszkiewicz, J; Wofsy, SC; Lin, JC; Gerbig, C; Longo, M; Freitas, S "Coupled weather research and forecasting-stochastic time-inverted lagrangian transport (WRF-STILT) model" METEOROLOGY AND ATMOSPHERIC PHYSICS , v.107 , 2010 , p.51 View record at Web of Science 10.1007/s00703-010-0068-

PROJECT OUTCOMES REPORT

Disclaimer

This Project Outcomes Report for the General Public is displayed verbatim as submitted by the Principal Investigator (PI) for this award. Any opinions, findings, and conclusions or recommendations expressed in this Report are those of the PI and do not necessarily reflect the views of the National Science Foundation; NSF has not approved or endorsed its content.

Collaborative Research: Improving Estimated Fluxes of Greenhouse Gases over North America Using a Receptor-Oriented Modeling Framework and In-situ Atmospheric Measurements

This study was intended to define how to determine rates of emission of important Greenhouse Gases and pollutants in urban areas and in areas of intensive agriculture, using measurements of concentrations of target gases (methane, carbon dioxide, carbon monoxide, nitrous oxide) in the atmosphere. In collaboration with our partners at AER, Inc, we constructed a very high resolution computer model to simulate the measurements made from tall towers in the Midwest, from aircraft in California, and ground based data from Salt Lake City and Boston. The results showed that emissions from agricultural areas were significantly larger than assumed in EPA inventories. We also showed that it is presently possible to detect changes in emissions over time from urban areas with a sensitivity of about 15%, almost good enough to use this approach as part of a compliance verification framework for regional and national Greenhouse Gas regulatory regimes. 

 

Three figures show examples.  Figure 1 a, b shows model results for the “dome” of CO2 over Salt Lake City, derived from automobiles and home heating/cooling, and the comparison of the model with observations in October, 2006 (Source: McKain, K., S. C. Wofsy, T. Nehrkorn, J. Eluszkiewicz, J. R. Ehleringer, and B. B. Stephens, Assessment of ground-based atmospheric observations for verification of greenhouse gas emissions from an urban region, Proc. Nat. Acad. Sci., doi 10.1073/pnas.1116645109, 2012).  Figure 2 shows the inferred spatial distribution of emissions for N2O (nitrous oxide) from agricultural regions of the US (Source: Miller, S., E. A. Kort, A. Hirsch, E. Dlugokencky, A. E. Andrews, A. Michalak, H. Tian, and S. C. Wofsy, Regional sources of nitrous oxide over the United States: Seasonal variation and spatial distribution, J. Geophys. Res. 117, D06310, doi:10.1029/2011JD016951, 2012).

 

 


Last Modified: 05/20/2012
Modified by: Steven C Wofsy