Award Abstract # 0711599
Collaborative Research: Properties of Melts and Supercooled Liquids at High Pressure by In Situ X-ray Computed Tomography and Absorption

NSF Org: EAR
Division Of Earth Sciences
Recipient: UNIVERSITY OF CALIFORNIA, DAVIS
Initial Amendment Date: February 7, 2008
Latest Amendment Date: February 7, 2008
Award Number: 0711599
Award Instrument: Standard Grant
Program Manager: Robin Reichlin
EAR
 Division Of Earth Sciences
GEO
 Directorate for Geosciences
Start Date: January 1, 2008
End Date: December 31, 2011 (Estimated)
Total Intended Award Amount: $360,937.00
Total Awarded Amount to Date: $360,937.00
Funds Obligated to Date: FY 2008 = $360,937.00
History of Investigator:
  • Charles Lesher (Principal Investigator)
    celesher@ucdavis.edu
Recipient Sponsored Research Office: University of California-Davis
1850 RESEARCH PARK DR STE 300
DAVIS
CA  US  95618-6153
(530)754-7700
Sponsor Congressional District: 04
Primary Place of Performance: University of California-Davis
1850 RESEARCH PARK DR STE 300
DAVIS
CA  US  95618-6153
Primary Place of Performance
Congressional District:
04
Unique Entity Identifier (UEI): TX2DAGQPENZ5
Parent UEI:
NSF Program(s): Petrology and Geochemistry,
Geophysics
Primary Program Source: 01000809DB NSF RESEARCH & RELATED ACTIVIT
Program Reference Code(s): 0000, 4444, OTHR
Program Element Code(s): 157300, 157400
Award Agency Code: 4900
Fund Agency Code: 4900
Assistance Listing Number(s): 47.050

ABSTRACT

The volumetric properties of non-crystalline materials relevant to Earth¹s interior are being studied using X-ray computed tomography and absorption at high pressures and temperatures. The results are applicable to differentiation of the magma ocean, core formation, and segregation and convection dynamics related to the thermal and chemical evolution of the Earth. The research utilizes the new rotating anvil apparatus and synchrotron X-ray radiation to determine density by volume reconstruction and from Beer-Lambert law using X-ray absorption data. The investigators focus their efforts on several simple and natural silicate melt compositions spanning a range of polymerization states, and on Fe-S-Ni-Si melts. Data acquired in this study improves constraints on the compressibility and thermal expansion required for an accurate equation of state for naturally occurring melt compositions. The project also includes technical improvements of tomography hardware on the 13-BM-D beamline operated by GSECARS - Advance Photon Source, Argonne National Laboratory, as well as, the development of new strategies for image acquisition at high P-T conditions and data processing with broader applications for non-destructive materials characterization.

PUBLICATIONS PRODUCED AS A RESULT OF THIS RESEARCH

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Gaudio, SJ; Sen, S; Lesher, CE "Pressure-induced structural changes and densification of vitreous MgSiO3" GEOCHIMICA ET COSMOCHIMICA ACTA , v.72 , 2008 , p.1222 View record at Web of Science 10.1016/j.gca.2007.12.00
Lesher, C.E. "Self-diffusion in silicate melts: Theory, observations and applications to magmatic systems" Reviews in Mineralogy and Geochemistry , v.72 , 2010 , p.269
Lesher, C.E., Wang, Y. ,Gaudio, S., Clark, A.N., and Rivers, M. "Volumetric properties of magnesium silicate glasses and supercooled liquid at high pressure by X-ray microtomography" Physics of the Earth and Planetary Interiors , v.174 , 2009 , p.292
Lesher, CE; Wang, Y; Gaudio, SJ; Clark, A; Sanehira, T; Yamada, A; Roberts, J "X-ray microtomography under extreme conditions" GEOCHIMICA ET COSMOCHIMICA ACTA , v.72 , 2008 , p.A536 View record at Web of Science
Schutt, D. and C.E. Lesher "Compositional trends among Kaapvaal Craton garnet peridotite xenoliths and their effects on seismic velocity and density" Earth Planet. Sci. Ltt , v.300 , 2010 , p.367
Wang, Y, Lesher, C, Fiquet, G, Rivers, ML, Nishiyama, N, Siebert, J, Roberts, J, Morard, G, Gaudio, S, Clark, A, Watson, H, Menguy, N, and Guyot, F "In situ high-pressure and high-temperature X-ray microtomographic imaging during large deformation: A new technique for studying mechanical behavior of multiphase composites" Geosphere , v.7 , 2011 , p.1 10.1130/GES00560.1
Yamada, A; Lesher, CE; Gaudio, SJ; Inoue, T; Funakoshi, K "Structure of MgSiO3 glass at high pressure and temperature" GEOCHIMICA ET COSMOCHIMICA ACTA , v.72 , 2008 , p.A1049 View record at Web of Science
Yamada, A., S.J. Gaudio, and C.E. Lesher "Densification of MgSiO3 glass with pressure and temperature" J. Phys.: Conf. Ser , v.215 , 2010 , p.012085 10.1088/1742-6596/215/1/012085

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