Award Abstract # 0425262
Influence of Global Sources on Free Tropospheric Ozone and Aerosols in the Western United States

NSF Org: AGS
Division of Atmospheric and Geospace Sciences
Recipient: UNIVERSITY OF WASHINGTON
Initial Amendment Date: August 2, 2004
Latest Amendment Date: August 2, 2004
Award Number: 0425262
Award Instrument: Standard Grant
Program Manager: Anne-Marie Schmoltner
AGS
 Division of Atmospheric and Geospace Sciences
GEO
 Directorate for Geosciences
Start Date: August 15, 2004
End Date: July 31, 2008 (Estimated)
Total Intended Award Amount: $609,233.00
Total Awarded Amount to Date: $609,233.00
Funds Obligated to Date: FY 2004 = $609,233.00
History of Investigator:
  • Daniel Jaffe (Principal Investigator)
    djaffe@u.washington.edu
Recipient Sponsored Research Office: University of Washington
4333 BROOKLYN AVE NE
SEATTLE
WA  US  98195-1016
(206)543-4043
Sponsor Congressional District: 07
Primary Place of Performance: University of Washington
4333 BROOKLYN AVE NE
SEATTLE
WA  US  98195-1016
Primary Place of Performance
Congressional District:
07
Unique Entity Identifier (UEI): HD1WMN6945W6
Parent UEI:
NSF Program(s): Atmospheric Chemistry
Primary Program Source: app-0104 
Program Reference Code(s): 0000, OTHR
Program Element Code(s): 152400
Award Agency Code: 4900
Fund Agency Code: 4900
Assistance Listing Number(s): 47.050

ABSTRACT

This project involves quantification of trace gases and aerosols with the goal to better define sources of these species contained in air masses transported to the western continental boundary of North America. The study will develop and make use of a new atmospheric measurement site on the summit of Mt. Bachelor in central Oregon. The 2.7 km altitude will likely enable regular sampling of free tropospheric air masses much as other mountain sites (for example, Mauna Loa Observatory, Hawaii, and Izana Atmospheric Observatory, Canary Islands). This will allow assessment of the contributions of long range transport of emissions to the regional budgets of ozone and fine particles.

During the study period, continuous measurements of ozone, carbon monoxide, and condensation nuclei concentrations, as well as aerosol light scattering efficiencies, will be made. During specific campaign periods, the measurement suite will be enhanced to include reactive nitrogen compounds (nitric oxide, nitrogen dioxide), peroxyacetyl nitrate (PAN), and the tracers of air mass origin, beryllium-7 and lead-210. Aircraft based concentration profiles of selected species and satellite based observations will be used to set the surface based measurements in horizontal and vertical context. A global chemical transport model will be used to help establish budgets and quantify the contributions from remote sources.

This project will establish a new atmospheric observing site at an altitude useful for atmospheric studies with a variety of goals. In this project, the data derived from the site will be useful for quantifying the role of long range transport on budgets of important tropospheric species such as ozone and fine particles. The project will also involve training of a post-doctoral research fellow and an undergraduate student. A community college faculty member will also be involved in the project.

PUBLICATIONS PRODUCED AS A RESULT OF THIS RESEARCH

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(Showing: 1 - 10 of 13)
Bertschi, I. T. & D. A. Jaffe "Long-range transport of ozone, carbon monoxide and aerosols to the NE Pacific Troposphere during the summer of 2003: Observations of smoke plumes from Asian Boreal fires." Journal of Geophysical Research , v.110 , 2005 , p.5135
Jaffe D. and Ray, J "Increase in Surface Ozone at Rural Sites in the Western U.S." Atmos.Enviro , 2007 doi: 10.1016/j.atmosenv.2007.02.03
Jaffe D. and Strode S. Sources "Fate and Transport of Atmospheric Mercury from Asia" Environ. Chem , v.5 , 2008 , p.121 doi:10.1071/EN08010
Jaffe, D., E. Prestbo, P. Swartzendruber, P. Weiss-Penzias, S. Kato, A. Takami, S. Hatakeyama, Y. Kajii "Export of atmospheric mercury from Asia" Atmospheric Environment , v.39 , 2005 , p.3029
Keating, T., J. West and D. Jaffe "Air Quality Impacts on Intercontinental Transport" EM , 2005 , p.28
Selin, NE; Jacob, DJ; Park, RJ; Yantosca, RM; Strode, S; Jaegle, L; Jaffe, D "Chemical cycling and deposition of atmospheric mercury: Global constraints from observations" JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES , v.112 , 2007 View record at Web of Science 10.1029/2006JD00745
Strode S., Jaeglé L., Jaffe D., Swartzendruber P., Selin N., Holmes C. and Yantosca R. "Trans-Pacific Transport of Mercury" . J.Geophys. Res , 2008 doi:10.1029/2007JD009428
Swartzendruber, P. C., D. A. Jaffe, D. Chand, J. A. Smith, L. Gratz, G. J. Keeler, S. Strode, L. Jaeglé, and C. Holmes "Vertical distribution of mercury, ozone, CO, and aerosol scatter in the Pacific Northwest during the spring of 2006 INTEX-B campaign" Journal of Geophysical Research , v.113 , 2008 doi:10.1029/2007JD009579
Swartzendruber, PC; Jaffe, DA; Prestbo, EM; Weiss-Penzias, P; Selin, NE; Park, R; Jacob, DJ; Strode, S; Jaegle, L "Observations of reactive gaseous mercury in the free troposphere at the Mount Bachelor Observatory" JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES , v.111 , 2006 View record at Web of Science 10.1029/2006JD00741
Weiss-Penzias, P., D. A. Jaffe, P. Swartzendruber, J. B. Dennison, D. Chand, W. Hafner, and E. Prestbo "Observations of Asian air pollution in the free tropospher at Mt. Bachelor Observatory in the spring of 2004" Journal of Geophysical Research , v.110 , 2006 , p.6522 doi: 10.1029/2005JD006522
Weiss-Penzias P., D. A. Jaffe, P. Swartzendruber, W. Hafner, D. Chand, and E. Prestbo "Quantifying Asian and biomass burning sources of mercury using the Hg/CO ratio in pollution plumes observed at the Mount Bachelor Observatory" Atmospheric Environment , v.41 , 2007 , p.4266 10.1016/j.atmosenv.2007.01.058
(Showing: 1 - 10 of 13)

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