Award Abstract # 1828420
MRI: Acquisition of a Magnetic Property Measurements System

NSF Org: DMR
Division Of Materials Research
Recipient: GEORGETOWN UNIVERSITY
Initial Amendment Date: August 6, 2018
Latest Amendment Date: August 6, 2018
Award Number: 1828420
Award Instrument: Standard Grant
Program Manager: Leonard Spinu
lspinu@nsf.gov
 (703)292-2665
DMR
 Division Of Materials Research
MPS
 Directorate for Mathematical and Physical Sciences
Start Date: August 15, 2018
End Date: July 31, 2021 (Estimated)
Total Intended Award Amount: $366,633.00
Total Awarded Amount to Date: $366,633.00
Funds Obligated to Date: FY 2018 = $366,633.00
History of Investigator:
  • Kai Liu (Principal Investigator)
    kai.liu@georgetown.edu
  • Sarah Stoll (Co-Principal Investigator)
  • Timothy Warren (Co-Principal Investigator)
  • Paola Barbara (Co-Principal Investigator)
  • Karah Knope (Co-Principal Investigator)
Recipient Sponsored Research Office: Georgetown University
MAIN CAMPUS
WASHINGTON
DC  US  20057
(202)625-0100
Sponsor Congressional District: 00
Primary Place of Performance: Georgetown University
37th & O St N W
Washington
DC  US  20057-1789
Primary Place of Performance
Congressional District:
00
Unique Entity Identifier (UEI): TF2CMKY1HMX9
Parent UEI: TF2CMKY1HMX9
NSF Program(s): Major Research Instrumentation
Primary Program Source: 01001819DB NSF RESEARCH & RELATED ACTIVIT
Program Reference Code(s):
Program Element Code(s): 118900
Award Agency Code: 4900
Fund Agency Code: 4900
Assistance Listing Number(s): 47.049

ABSTRACT

This Major Research Instrumentation award will provide support for the acquisition of a state-of-the-art magnetometer that combines extreme sensitivity with multiple measurement modes. The instrument will meet a critical need for cutting-edge magnetic characterization, particularly for a wide variety of functional magnetic and superconducting nanostructures, on the Georgetown campus and in the greater District of Columbia area. The research projects that will be enabled by this instrument have potentially major technological impacts in low power nanoelectronics, quantum computation, magnetic recording, magnetic semiconductors, nanophotonics, catalysis and bioinorganic chemistry, magnetic resonance imaging, and hyperthermia therapeutics. The instrument will have a strong impact on broadening participation of underrepresented groups in STEM fields from a broad user base at Georgetown and nearby institutions. It will also be utilized to provide research experience for undergraduate students through several partner REU programs.


This Major Research Instrumentation award support the acquisition of a Magnetic Property Measurement System (MPMS3), with unique technical features that are critical to support many current and future research efforts at Georgetown University. The extreme sensitivity, wide magnetic field range and temperature span, versatile operation modes, and cryogen-free capability are essential for studying a wide variety of technologically important magnetic and superconducting materials. The interdisciplinary research projects that will be enabled by this instrument include topological spin textures, chiral Majorana fermions, next generation heat-assisted magnetic recording media, single-molecule magnets, magnetic semiconductors, biomedical applications of magnetic nanoparticles, structure-property relationships in f-element materials, paramagnetic molecular complexes in catalysis and bioinorganic chemistry, and molecular spintronics based computational and memory devices. The instrument will be integrated with graduate and undergraduate curriculum to provide students with hands-on learning experiences, and promote teaching, learning and training.

This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

PUBLICATIONS PRODUCED AS A RESULT OF THIS RESEARCH

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(Showing: 1 - 10 of 19)
de Rojas, Julius and Quintana, Alberto and Lopeandía, Aitor and Salguero, Joaquín and Muñiz, Beatriz and Ibrahim, Fatima and Chshiev, Mairbek and Nicolenco, Aliona and Liedke, Maciej O. and Butterling, Maik and Wagner, Andreas and Sireus, Veronica and Aba "Voltage-driven motion of nitrogen ions: a new paradigm for magneto-ionics" Nature Communications , v.11 , 2020 https://doi.org/10.1038/s41467-020-19758-x Citation Details
Beeson, W B and Bista, D and Zhang, H R and Krylyuk, S and Bhattacharya, D and Naushin, N and Kukreja, R and Davydov, A V and Yin, G and Liu, Kai "Single Phase $L1_{0}$-Ordered High Entropy Thin Films with High Magnetic Anisotropy" , 2024 https://doi.org/10.1109/TMRC62973.2024.10713986 Citation Details
Beeson, Willie B and Bista, Dinesh and Naushin, Nushrat and N'Diaye, Alpha T and Kukreja, Roopali and Yin, Gen and Liu, Kai "Switching of Magnetic Order via NonMagnetic Al Addition in FeCoNiMnAl x Films" Advanced Functional Materials , 2025 https://doi.org/10.1002/adfm.202424741 Citation Details
Beeson, Willie B and Bista, Dinesh and Zhang, Huairuo and Krylyuk, Sergiy and Davydov, Albert V and Yin, Gen and Liu, Kai "SinglePhase L 1 0 Ordered High Entropy Thin Films with High Magnetic Anisotropy" Advanced Science , 2024 https://doi.org/10.1002/advs.202308574 Citation Details
Bista, Dinesh and Beeson, Willie B and Sengupta, Turbasu and Jackson, Jerome and Khanna, Shiv N and Liu, Kai and Yin, Gen "Fast ab initio design of high-entropy magnetic materials" Physical Review Materials , v.9 , 2025 https://doi.org/10.1103/PhysRevMaterials.9.L031401 Citation Details
Chen, Zhijie and Jensen, Christopher_J and Liu, Chen and Liu, Yijing and Kinane, Christy_J and Caruana, Andrew_John and Grutter, Alexander_J and Borchers, Julie_A and Zhang, Xixiang and Liu, Kai "Reconfigurable All-Nitride Magneto-Ionics" ACS Nano , 2025 https://doi.org/10.1021/acsnano.5c04013 Citation Details
Chen, Zhijie and Jensen, Christopher J. and Liu, Chen and Zhang, Xixiang and Liu, Kai "Ionically driven synthesis and exchange bias in Mn4N/MnN <i>x</i> heterostructures" Applied Physics Letters , v.123 , 2023 https://doi.org/10.1063/5.0165895 Citation Details
Garskaite, Edita and Stoll, Sarah L. and Forsberg, Fredrik and Lycksam, Henrik and Stankeviciute, Zivile and Kareiva, Aivaras and Quintana, Alberto and Jensen, Christopher J. and Liu, Kai and Sandberg, Dick "The Accessibility of the Cell Wall in Scots Pine ( Pinus sylvestris L.) Sapwood to Colloidal Fe 3 O 4 Nanoparticles" ACS Omega , v.6 , 2021 https://doi.org/10.1021/acsomega.1c03204 Citation Details
Jensen, Christopher J. and Quintana, Alberto and Quarterman, Patrick and Grutter, Alexander J. and Balakrishnan, Purnima P. and Zhang, Huairuo and Davydov, Albert V. and Zhang, Xixiang and Liu, Kai "Nitrogen-Based Magneto-ionic Manipulation of Exchange Bias in CoFe/MnN Heterostructures" ACS Nano , v.17 , 2023 https://doi.org/10.1021/acsnano.2c12702 Citation Details
Jensen, Christopher J. and Quintana, Alberto and Sall, Mamour and Diez, Liza Herrera and Zhang, Junwei and Zhang, Xixiang and Ravelosona, Dafiné and Liu, Kai "Ion irradiation and implantation modifications of magneto-ionically induced exchange bias in Gd/NiCoO" Journal of Magnetism and Magnetic Materials , v.540 , 2021 https://doi.org/10.1016/j.jmmm.2021.168479 Citation Details
Lo Conte, Roberto and Nandy, Ashis K. and Chen, Gong and Fernandes Cauduro, Andre L. and Maity, Ajanta and Ophus, Colin and Chen, Zhijie and NDiaye, Alpha T. and Liu, Kai and Schmid, Andreas K. and Wiesendanger, Roland "Tuning the Properties of Zero-Field Room Temperature Ferromagnetic Skyrmions by Interlayer Exchange Coupling" Nano Letters , v.20 , 2020 10.1021/acs.nanolett.0c00137 Citation Details
(Showing: 1 - 10 of 19)

PROJECT OUTCOMES REPORT

Disclaimer

This Project Outcomes Report for the General Public is displayed verbatim as submitted by the Principal Investigator (PI) for this award. Any opinions, findings, and conclusions or recommendations expressed in this Report are those of the PI and do not necessarily reflect the views of the National Science Foundation; NSF has not approved or endorsed its content.

Acquisition and installation of a Magnetic Property Measurement System (MPMS3) system have been completed in this project. The instrument is a state-of-the-art magnetometer that combines the extreme sensitivity of a Superconducting QUantum Interference Device (SQUID) with multiple measurement modes. It meets a critical need for cutting-edge magnetic characterization, particularly for a wide variety of functional magnetic nanostructures, on the Georgetown campus and in the greater Washington, DC area.

 

Intellectual Merit

The MPMS3 instrument has unique technical features that are critical to support many NSF-funded projects as well as other research efforts: its extreme sensitivity allows measurement of magnetic nanoparticles, nanowires, and ultrathin films with the smallest dimensions; the wide magnetic field range and temperature span, versatile operation modes, and cryogen-free Evercool capability are essential for studying a wide variety of technologically important magnetic and superconducting materials.

A broad range of ground-breaking interdisciplinary research projects have been enabled by this instrument. For example, we have demonstrated that interlayer exchange coupling between a reference and a free magnet can be used to stabilize a whirling magnetic configuration known as skyrmions, at room temperature and without any magnetic field, which are promising for low dissipation information storage; we have probed magnetic interactions in thermoelectric composite materials with micron-sized as well as nanoscale magnetic inclusions, and illustrated how the microstructures correlate with improved power factor and mechanical properties for applications in sustainable energy conversion; we have demonstrated the mechanisms for a newly developed two-way magnetic resonance tuning (TMRET) imaging technique that has profound impacts in improving magnetic resonance imaging (MRI) sensitivity and early cancer detection; we have revealed microscopic mechanisms of ionic migrations across buried interfaces and how they can be employed to electrically manipulate the magnetic responses, leading to novel concepts of energy-efficient nanoelectronic devices; we have also illustrated how magnetic nanoparticles can be infiltrated into cell walls of Scots pine sapwood and add additional functionalities.

 

Broader Impacts

This shared MPMS3 system has had major impacts for the research infrastructure at Georgetown University. It has provided urgently needed capabilities for magnetic characterizations. There is also a broad and growing user base from nearby institutions. The research projects that have been enabled by this instrument have potentially major technological impacts in low dissipation nanoelectronics, magneto-ionics, sustainable energy conversion, next generation magnetic recording media, magnetic resonance imaging, and bio-based functional materials. The results have been broadly disseminated through peer-reviewed publications, including several in high-impact journals in the field, and through many invited and contributed talks at conferences and research institutions. This instrument has had a strong impact on broadening participation of underrepresented groups in STEM fields. The instrument has been integrated with graduate and undergraduate curriculum to provide students with hands-on learning experiences. It has also been utilized to provide research experience for undergraduate students through local REU programs. 


Last Modified: 12/21/2021
Modified by: Kai Liu

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